Ignatyuk A.V.1, Lunev V.P.1, Shubin Yu.N.1, Gai E.V.1, Titarenko N.N.1, Gudowski W.2
Investigations aimed at the development of neutron cross section evaluations for actinides performed at IPPE in collaboration with Royal Institute of Technology, Stockholm at intermediate energies in the range of 0–200 MeV are briefly described on the example of 239Pu. The coupled-channels optical model is used to calculate the neutron total, elastic and reaction cross sections and the elastic scattering angular distributions. Evaluations of the neutron and charged particle emission cross sections and of the fission cross sections are obtained on the basis of the statistical description that includes direct, preequilibrium and equilibrium mechanisms of nuclear reactions. The Kalbach parametrization of angular distributions is used to describe the double-differential cross sections of emitted neutrons and charged particles in ENDF/B-VI format. These investigations resulted in creation of complete neutron and proton data files for 238U and 232Th and neutron data file for 239Pu up to 150 MeV. These files were processed with NJOY.
1. A.J.Koning, Requirements for an Evaluated Nuclear Data File for Accelerator Based Transmutation,
Report NEA/NSC/DOC(93)6 and ECN-C-93-005; Nuclear Data Evaluation for Accelerator-Driven
Systems, in Proc. Second International Conference on Accelerator-Driven Transmutation Technologies
and Applications, Kalmar, Sweden, June 3-7, 1996, Vol. 1, p. 438, H. Condé, Ed., Gotab, Stockholm,
Sweden (1997).
2. H.W.Bertini, Phys.Rev. 188, 1711 (1969).
3. T.W.Armstrong, K.C.Chandler, Nucl. Sci. Eng. 49, 110 (1972).
4. V.S.Barashenkov, V.D.Toneev, Interactions of High Energy Particles with Nuclei (Atomizdat, Moscow,
1972).
5. R.E.Prael, H.Lichtenstein, Users Guide to the LAHET Code System, Report LA-UR-89-3014, Los
Alamos National Laboratory (1989).
6. M.B.Chadwick, P.G.Young, S.Chiba, S.C. Frankle, G.M. Hale, H.G. Hughes, A.J. Koning, R.C. Little,
R.E. MacFarlane, R.E. Prael, and L.S. Waters, Nucl. Sci. Eng. 131, 293 (1999).
7. P.G.Young, E.D.Arthur, M.B.Chadwick, Comprehensive Nuclear Model Calculations: Theory and Use
of the GNASH Code. in Proc.IAEA Workshop on Nuclear Reaction Data and Nuclear Reactors Trieste,
Italy, 15 April - 17 May 1996, Vol. 1, p. 227, A.Gandini and G.Reffo Editors, World Scientific,
Singapore (1998).
8. A.V.Ignatyuk, Level Densities. In: Reference Input Parameter Library for Nuclear Model Calculations -
Handbook, IAEA - TECDOC-1034, Vienna, 1998, ch. 5.
9. L.F.Hansen, B.A.Pohl, C.Wong, R.C.Haight, Ch.Lagrange, Phys. Rev. C34, 2075 (1986).
10. V.A.Konshin, Calculations of Neutron and Proton Induced Reaction Cross-sections for Actinides in the
Energy Region from 10 MeV to 1 GeV. Report JAERI-Research-95-036, Japan Atomic Energy
Research Institute (1995).
11. P.G.Young, Optical Model Parameters. In Reference Input Parameter Library for Nuclear Model
Calculations - Handbook, IAEA-TECDOC-1034, Vienna, 1998, ch. 4.
12. H.Vonach, A.Pavlik, M.B.Chadwick, R.C.Haight, R.O.Nelson, S.A.Wender, and P.G.Young, Phys.
Rev. C50, 1952 (1994).
13. M.B.Chadwick, P.G.Young, GNASH Calculations of the Neutron and Proton Induced Reactions for
Lead Isotopes and Benchmarking of Results. Report T-2-96, Los Alamos National Laboratory (1996).
14. V.S.Barashenkov, Cross-sections of Particle and Nucleus Interactions with Nuclei (Russian), JINR,
Dubna, 1993.
15. F.Hansen, B.A.Pohl, C.Wong, R.C.Haight, Ch.Lagrange, Phys. Rev. C34, 2075 (1986).
16. R.L.Henkel, Report LA-1493, (1952).
17. K.A.Nadolny, K.A.Green, P.Stoler, Total Neutron Cross-section of 239-Pu. Preprint USNDC-9, 170
(1973).
18. J.M.Peterson, A.Bratenahl, J.P.Stoering, Phys.Rev. v.120 (1960) p.1252.
19. W.P.Poenitz, J.F.Whalen, Neutron Total Cross-section Measurements in the Energy Region from 47
keV to 20 MeV. Report ANL-NDM-80, (1983).
20. R.K.Smith, R.K.Henkel, R.A.Noble, BAP 2,(1957).
21. P.Staples, and K.Morley, Nucl.Sci.Eng. v.129 (1998) p.149.
22. K.,Kari and S.Cieriacks, Measurements of Neutron Induced Fission Cross-section Ratios at the
Karlsruhe Isochronous Cyclotron. Report EANDC(E)-157, 8, BNL (1978).
23. P.W.Lisowski, J.L.Ullman, S.J.Balestrini, A.D.Carlson, O.A.Wasson, N.W.Hill, in: Proc. of Int. Conf.
On Nuclear Data for Science and Technology. Mito, Japan, May 30-June 3. (Ed. I. Igarasi) (1988) p.97.
24. P.W.Lisowski et al., in Proc. Symp. on Neutron Cross-Sections from 10 to 50 MeV. Upton, 1980, Vol.
1, p.301; in Proc. Specialists' Meeting on Neutron Cross-Sections Standards for the Energy Region
above 20 MeV (Uppsala, May 1991), NEANDC-305/U, p.177 (1991).
25. A.Yu.Donets, A.V.Evdokimov, A.V.Fomichev, T.Fukahori, A.B.Laptev, G.A.Petrov,
O.A.Shcherbakov, Yu.V.Tuboltsev, A.S.Vorobyev, Neutron Induced Fission Cross-Sections of 233U,
235U, 238U, 232Th, 239Pu, and 237Np in the Energy Range 1 - 200 MeV. In: Proceedings of VII
International Seminar on Interaction Neutrons with Nuclei, (Dubna, 1999, to be publ.)
26. A.V.Ignatyuk, G.A.Kudyaev, A.R.Junghans, M.deJong, M.G.Clerc, and K.H.Schmidt, Nucl. Phys.
A593, 519 (1995).
27. J.Fréhaut, "Nu-bar Results at Bruyères-le-Châtel", Private communication to EXFOR-21685 (1976).
28. C.Kalbach, F.M.Mann. Phys. Rev. C23, 112 (1981).
29. J.Bojowald, H.Machner, H.Nann, W.Oelert, M.Rogge, and P.Turek, Phys. Rev. C38, 1153 (1988).
30. F.D.Becchetti Jr, and G.W.Greenlees, Ann. Rep. J.H. Williams Lab., Univ. Minnesota (1969).
31. V.Avrigeanu, P.E.Hodgson, and M.Avrigeanu, Phys.Rev. C49, 2255 (1994).
32. A.Iwamoto, K.Harada, Phys. Rev. C26, 1821 (1982).
33. A.I.Dityuk, A.Yu.Konobeyev, V.P.Lunev, Yu.N.Shubin, New Advanced Version of Computer Code
ALICE-IPPE, Report INDC(CCP)-410, IAEA, Vienna (1998).
34. C.Kalbach, F.M.Mann, “Phenomenology of Continuum Angular Distributions. I. Systematics and
Parameterization,” Phys. Rev. C23, 112 (1981).